MPI-FKF homepage > Keimer's department

Physics of strongly correlated electron systems

Our department uses neutron and x-ray diffraction and spectroscopy, optical spectroscopy, and Raman scattering, supported by various supplementary methods, to explore the structure and dynamics of materials with strong electron correlations. Topics of particular current interest include the interplay between spin, charge, and orbital degrees of freedom in transition metal oxides; mechanisms of unconventional superconductivity in solids; and quantum many-body physics at oxide interfaces. We strongly believe that close collaboration between experimentalists and theorists is essential for progress in this field. To facilitate this interaction, a small theory group operates within the department. We also have a strong effort in the development of new spectroscopic methods, especially spectral ellipsometry with synchrotron radiation and neutron resonance spin-echo spectroscopy. To this end, we operate experimental facilities at the ANKA synchrotron in Karlsruhe and at the FRM-II research reactor in Garching, in addition to our in-house laboratories. The recently commissioned TRISP spectrometer at the FRM-II allows the determination of the lifetimes of collective excitations in solids with unprecedented accuracy.

Our research projects

Unconventional superconductivity

The microscopic description of superconductivity in complex materials such as layered cuprates, cobaltates, or the recently discovered iron pnictides, is one of the most important challenges in current solid-state physics. Our group uses high-quality single crystals and state-of-the-art experimental methods to derive accurate spectra of spin and charge excitations in these materials. Such data are essential to motivate and test new theoretical concepts for the correlated electron systems that support unconventional superconductivity.

Low-dimensional magnetism

The discovery of high-temperature superconductivity has stimulated a tremendous upsurge of interest in the quantitative understanding of low-dimensional quantum magnets. Experiments performed in our group elucidate the magnetic structure and dynamics of one- and two-dimensional magnets and their influence on charge transport. Novel compounds synthesized by chemists at our institute are of particular importance.

Orbital physics

The exceptionally rich phase behavior observed in transition metal oxides originates in a competition between many-body states with different spin, orbital, and charge ordering patterns. Work in our group seeks to unravel the microscopic mechanisms underlying this competition. To this end, spectroscopic data on orbitally degenerate transition metal oxides obtained in our group are analyzed and interpreted in close collaboration with theorists.

Oxide heterostructures

Carefully controlled interfaces between two materials can give rise to novel physical phenomena and functionalities not exhibited by either of the constituent materials alone. Modern synthesis methods have yielded high-quality heterostructures and superlattices of oxide materials with competing quantum many-body states. In order to explore new correlation-driven interface phenomena, our group seeks to understand and manipulate the spin and orbital polarization at oxide interfaces (“orbital engineering”).
Recent highlights

Emergent phenomena at oxide interfaces

A review article in Nature Materials discusses recent advances in understanding novel interface states that arise in oxide heterostructures due to the charge, spin and orbital reconstruction effects.  
H. Y. Hwang et al., Nature Materials, 2012

Magnetic resonant mode in the Rb2Fe4Se5 superconductor

A resonant magnetic excitation in the Rb-245 iron-selenide superconductor has been discovered at a wave vector, which differs from the ones characterizing magnetic resonant modes in other iron-based superconductors. 
J. T. Park et al. Phys. Rev. Lett., 2011

Intense high-energy paramagnons in high-Tc superconductors

Damped spin excitations are found in a large family of high-Tc superconductors by resonant inelastic x-ray scattering. Their dispersions and spectral weights are similar to those of magnons in undoped cuprates.  
M. Le Tacon et al., Nature Physics, 2011

Dimensionality Control of Phase Transitions in Superlattices

Results of optical ellipsometry and muon spin rotation on LaNiO3/LaAlO3 multilayers demonstrate that the dimensionality and electronic order in these systems can be controlled by varying the thickness of the LaNiO3 layer.  
A. V. Boris et al., Science, 2011

Superconductivity-induced optical anomaly in an iron arsenide

Spectroscopic ellipsometry reveals that excitations with energies up to two orders of magnitude greater than the energy gap are affected by the superconducting transition in the multiband metal Ba0.68K0.32Fe2As2.  
A. Charnukha et al., Nature Communications, 2011

Orbital reflectometry

We introduce a new experimental method that yields quantitative, depth-resolved orbital polarization profiles of metal-oxide multilayers with a resolution of one atomic unit cell. That is, it can tell within an accuracy of a few percent which d-orbitals are occupied in which atomic layer.  
E. Benckiser et al., Nature Materials, 2011